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Author Sakiko Ishino, Shohei Hattori, Joel Savarino, Bruno Jourdain, Susanne Preunkert, Michel Legrand, Nicolas Caillon, Albane Barbero, Kota Kuribayashi, Naohiro Yoshida
Title Seasonal variations of triple oxygen isotopic compositions of atmospheric sulfate, nitrate, and ozone at Dumont d'Urville, coastal Antarctica Type Journal
Year 2017 Publication Atmospheric Chemistry and Physics Abbreviated Journal
Volume 17 Issue 5 Pages 3713-3727
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Abstract
Programme 1177
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Address
Corporate Author Thesis
Publisher Place of Publication Editor
Language Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 1680-7316 ISBN 1680-7316 Medium
Area Expedition Conference
Notes Approved yes
Call Number Serial 7349
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Author Sprovieri, F., Pirrone, N., Bencardino, M., D'Amore, F., Angot, H., Barbante, C., Brunke, E.G., Arcega-Cabrera, F., Cairns, W., Comero, S., Diéguez, M.D.C., Dommergue, A., Ebinghaus, R., Feng, X.B., Fu, X., Garcia, P.E., Gawlik, B.M., Hageström, U., Hansson, K., Horvat, M., Kotnik, J., Labuschagne, C., Magand, O., Martin, L., Mashyanov, N., Mkololo, T., Munthe, J., Obolkin, V., Islas, M.R., Sena, F., Somerset, V., Spandow, P., Vardè, M., Walters, C., Wängberg, I., Weigelt, A., Yang, X., Zhang, H.
Title Five-year records of Total Mercury Deposition flux at GMOS sites in the Northern and Southern Hemispheres. Type Journal Article
Year 2016 Publication Atmos. chem. phys. Abbreviated Journal
Volume 17 Issue 4 Pages 2689-2708
Keywords
Abstract
Programme 1028
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Address
Corporate Author Thesis
Publisher Place of Publication Editor
Language Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 1680-7324 ISBN Medium
Area Expedition Conference
Notes Approved yes
Call Number Serial 6558
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Author
Title Five-year records of mercury wet deposition flux at GMOS sites in the Northern and Southern hemispheres Type Journal
Year 2017 Publication Atmos. chem. phys. Abbreviated Journal
Volume 17 Issue 4 Pages 2689-2708
Keywords
Abstract
Programme 1028
Campaign
Address
Corporate Author Thesis
Publisher Place of Publication Editor
Language Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 1680-7324 ISBN 1680-7324 Medium
Area Expedition Conference
Notes Approved yes
Call Number Serial 6588
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Author
Title Particulate-phase mercury emissions from biomass burning and impact on resulting deposition: a modelling assessment Type Journal
Year 2017 Publication Atmos. chem. phys. Abbreviated Journal
Volume 17 Issue 3 Pages 1881-1899
Keywords
Abstract Mercury (Hg) emissions from biomass burning (BB) are an important source of atmospheric Hg and a major factor driving the interannual variation of Hg concentrations in the troposphere. The greatest fraction of Hg from BB is released in the form of elemental Hg (Hg0(g)). However, little is known about the fraction of Hg bound to particulate matter (HgP) released from BB, and the factors controlling this fraction are also uncertain. In light of the aims of the Minamata Convention to reduce intentional Hg use and emissions from anthropogenic activities, the relative importance of Hg emissions from BB will have an increasing impact on Hg deposition fluxes. Hg speciation is one of the most important factors determining the redistribution of Hg in the atmosphere and the geographical distribution of Hg deposition. Using the latest version of the Global Fire Emissions Database (GFEDv4.1s) and the global Hg chemistry transport model, ECHMERIT, the impact of Hg speciation in BB emissions, and the factors which influence speciation, on Hg deposition have been investigated for the year 2013. The role of other uncertainties related to physical and chemical atmospheric processes involving Hg and the influence of model parametrisations were also investigated, since their interactions with Hg speciation are complex. The comparison with atmospheric HgP concentrations observed at two remote sites, Amsterdam Island (AMD) and Manaus (MAN), in the Amazon showed a significant improvement when considering a fraction of HgP from BB. The set of sensitivity runs also showed how the quantity and geographical distribution of HgP emitted from BB has a limited impact on a global scale, although the inclusion of increasing fractions HgP does limit Hg0(g) availability to the global atmospheric pool. This reduces the fraction of Hg from BB which deposits to the world's oceans from 71 to 62?%. The impact locally is, however, significant on northern boreal and tropical forests, where fires are frequent, uncontrolled and lead to notable Hg inputs to local ecosystems. In the light of ongoing climatic changes this effect could be potentially be exacerbated in the future.
Programme 1028
Campaign
Address
Corporate Author Thesis
Publisher Place of Publication Editor
Language Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 1680-7324 ISBN 1680-7324 Medium
Area Expedition Conference
Notes Approved yes
Call Number Serial 6590
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Author Michel Legrand, Susanne Preunkert, Eric Wolff, Rolf Weller, Bruno Jourdain, Dietmar Wagenbach
Title Type Journal
Year 2017 Publication Atmospheric Chemistry and Physics Abbreviated Journal
Volume 17 Issue 22 Pages 14039-14054
Keywords
Abstract
Programme 414
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Address
Corporate Author Thesis
Publisher Place of Publication Editor
Language Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 1680-7316 ISBN 1680-7316 Medium
Area Expedition Conference
Notes Approved yes
Call Number Serial 7311
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Author
Title Type Journal
Year 2017 Publication Atmos. Chem. Phys. Abbreviated Journal
Volume 17 Issue 18 Pages 11135-11161
Keywords
Abstract
Programme 416
Campaign
Address
Corporate Author Thesis
Publisher Place of Publication Editor
Language Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 1680-7324 ISBN 1680-7324 Medium
Area Expedition Conference
Notes Approved yes
Call Number Serial 6971
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Author Casado M, Landais A, Masson-Delmotte V, Genthon C, Kerstel E, Kassi S, Arnaud L, Picard G, Prie F, Cattani O, Steen-Larsen H-C, Vignon E, Cermak P,
Title Continuous measurements of isotopic composition of water vapour on the East Antarctic Plateau Type Journal Article
Year 2016 Publication ATMOSPHERIC CHEMISTRY AND PHYSICS Abbreviated Journal
Volume 16 Issue 13 Pages 8521-8538
Keywords
Abstract
Programme 1110
Campaign
Address
Corporate Author Thesis
Publisher Place of Publication Editor
Language Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 1680-7324 ISBN Medium
Area Expedition Conference
Notes Approved yes
Call Number Serial 6429
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Author Angot, H., Dion, I., Vogel, N., Legrand, M., Magand, O., Dommergue, A.
Title Multi-year record of atmospheric mercury at Dumont d'Urville, East Antarctic coast: continental outflow and oceanic influences Type Journal Article
Year 2016 Publication Atmospheric chemistry and physics Abbreviated Journal 1680-7316
Volume 16 Issue 13 Pages 8265-8279
Keywords
Abstract Under the framework of the Global Mercury Observation System (GMOS) project, a 3.5-year record of atmospheric gaseous elemental mercury (Hg(0)) has been gathered at Dumont d'Urville (DDU, 66°40′ S, 140°01′ E, 43 m above sea level) on the East Antarctic coast. Additionally, surface snow samples were collected in February 2009 during a traverse between Concordia Station located on the East Antarctic plateau and DDU. The record of atmospheric Hg(0) at DDU reveals particularities that are not seen at other coastal sites: a gradual decrease of concentrations over the course of winter, and a daily maximum concentration around midday in summer. Additionally, total mercury concentrations in surface snow samples were particularly elevated near DDU (up to 194.4 ng L−1) as compared to measurements at other coastal Antarctic sites. These differences can be explained by the more frequent arrival of inland air masses at DDU than at other coastal sites. This confirms the influence of processes observed on the Antarctic plateau on the cycle of atmospheric mercury at a continental scale, especially in areas subject to recurrent katabatic winds. DDU is also influenced by oceanic air masses and our data suggest that the ocean plays a dual role on Hg(0) concentrations. The open ocean may represent a source of atmospheric Hg(0) in summer whereas the sea-ice surface may provide reactive halogens in spring that can oxidize Hg(0). This paper also discusses implications for coastal Antarctic ecosystems and for the cycle of atmospheric mercury in high southern latitudes.
Programme 1028
Campaign
Address
Corporate Author Thesis
Publisher Place of Publication Editor
Language Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 1680-7316 ISBN Medium
Area Expedition Conference
Notes Approved yes
Call Number Serial 6562
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Author H. Angot, I. Dion, N. Vogel, M. Legrand, O. Magand, A. Dommergue
Title Multi-year record of atmospheric mercury at Dumont d'Urville, East Antarctic coast: continental outflow and oceanic influences Type Journal
Year 2016 Publication Atmos. chem. phys. Abbreviated Journal
Volume 16 Issue 13 Pages 8265-8279
Keywords
Abstract
Programme 1028
Campaign
Address
Corporate Author Thesis
Publisher Place of Publication Editor
Language Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 1680-7324 ISBN 1680-7324 Medium
Area Expedition Conference
Notes Approved yes
Call Number Serial 6594
Permanent link to this record
 

 
Author Angot, H., Magand, O., Helmig, D., Ricaud, P., Quennehen, B., Gallée, H., Del Guasta, M., Sprovieri, F., Pirrone, N., Savarino, J., and Dommergue, A.
Title New insights into the atmospheric mercury cycling in central Antarctica and implications on a continental scale Type Journal Article
Year 2016 Publication ATMOSPHERIC CHEMISTRY AND PHYSICS Abbreviated Journal
Volume 16 Issue 13 Pages 8249-8264
Keywords
Abstract Under the framework of the GMOS project (Global Mercury Observation System) atmospheric mercury monitoring has been implemented at Concordia Station on the high-altitude Antarctic plateau (75°06′?S, 123°20′?E, 3220?m above sea level). We report here the first year-round measurements of gaseous elemental mercury (Hg(0)) in the atmosphere and in snowpack interstitial air on the East Antarctic ice sheet. This unique data set shows evidence of an intense oxidation of atmospheric Hg(0) in summer (24-hour daylight) due to the high oxidative capacity of the Antarctic plateau atmosphere in this period of the year. Summertime Hg(0) concentrations exhibited a pronounced daily cycle in ambient air with maximal concentrations around midday. Photochemical reactions and chemical exchange at the air–snow interface were prominent, highlighting the role of the snowpack on the atmospheric mercury cycle. Our observations reveal a 20 to 30?% decrease of atmospheric Hg(0) concentrations from May to mid-August (winter, 24?h darkness). This phenomenon has not been reported elsewhere and possibly results from the dry deposition of Hg(0) onto the snowpack. We also reveal the occurrence of multi-day to weeklong atmospheric Hg(0) depletion events in summer, not associated with depletions of ozone, and likely due to a stagnation of air masses above the plateau triggering an accumulation of oxidants within the shallow boundary layer. Our observations suggest that the inland atmospheric reservoir is depleted in Hg(0) in summer. Due to katabatic winds flowing out from the Antarctic plateau down the steep vertical drops along the coast and according to observations at coastal Antarctic stations, the striking reactivity observed on the plateau most likely influences the cycle of atmospheric mercury on a continental scale.
Programme 910
Campaign
Address
Corporate Author Thesis
Publisher Place of Publication Editor
Language Summary Language Original Title
Series Editor Series Title Abbreviated Series Title
Series Volume Series Issue Edition
ISSN 1680-7316 ISBN Medium
Area Expedition Conference
Notes Approved yes
Call Number Serial 6446
Permanent link to this record