| |
Records |
Links |
|
Author |
Florent Domine |
|
| |
Title |
Can We Monitor Snow Properties on Sea Ice to Investigate Its Role in Tropospheric Ozone Depletion? |
Type |
Journal |
| |
Year |
2017 |
Publication |
Journal of Geophysical Research: Atmospheres |
Abbreviated Journal |
|
|
| |
Volume |
122 |
Issue |
20 |
Pages |
11,107-11,111 |
|
| |
Keywords |
Arctic bromine ozone snow troposphere |
|
| |
Abstract |
In the lower troposphere over the Arctic Ocean, ozone is often destroyed in spring by chemical chain reactions involving the reactive bromine species Br and BrO. The role of surface snow in generating reactive bromine has been suspected, but many details of the processes not understood. Using unique data such as BrO concentrations from instruments on buoys, Burd et al. (2017, https://doi.org/10.1002/2017JD026906) observed that the snowmelt onset date often coincides with the end of the reactive bromine season. They proposed that the decrease in snow-specific surface area and/or the occurrence of liquid water in snow induced by melting dramatically slows the rate of surface reactions generating bromine, indicating that the physical state of the snow is critical for bromine generation. Their suggestion is discussed, and a method to test it using novel instrumentation recently available is proposed. |
|
| |
Programme |
1042 |
|
| |
Campaign |
|
|
| |
Address |
|
|
| |
Corporate Author |
|
Thesis |
|
|
| |
Publisher |
|
Place of Publication |
|
Editor |
|
|
| |
Language |
|
Summary Language |
|
Original Title |
|
|
| |
Series Editor |
|
Series Title |
|
Abbreviated Series Title |
|
|
| |
Series Volume |
|
Series Issue |
|
Edition |
|
|
| |
ISSN  |
2169-8996 |
ISBN |
2169-8996 |
Medium |
|
|
| |
Area |
|
Expedition |
|
Conference |
|
|
| |
Notes |
|
Approved |
yes |
|
| |
Call Number |
|
Serial |
7464 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
F. Lemonnier, J.-B. Madeleine, C. Claud, C. Palerme, C. Genthon, T. L'Ecuyer, N. B. Wood |
|
| |
Title |
CloudSat-Inferred Vertical Structure of Snowfall Over the Antarctic Continent |
Type |
Journal |
| |
Year |
2019 |
Publication |
Journal of Geophysical Research: Atmospheres |
Abbreviated Journal |
|
|
| |
Volume |
125 |
Issue |
2 |
Pages |
e2019JD031399 |
|
| |
Keywords |
Antarctica climatology CloudSat cloud-profiling radar precipitation snowfall vertical structure |
|
| |
Abstract |
Current global warming is causing significant changes in snowfall in polar regions, directly impacting the mass balance of the ice caps. The only water supply in Antarctica, precipitation, is poorly estimated from surface measurements. The onboard cloud-profiling radar of the CloudSat satellite provided the first real opportunity to estimate solid precipitation at continental scale. Based on CloudSat observations, we propose to explore the vertical structure of precipitation in Antarctica over the 2007–2010 period. A first division of this data set following a topographical approach (continent vs. peripheral regions, with a 2,250 m topographical criterion) shows a high snowfall rate (275 mm yr at 1,200 m above ground level) with low relative seasonal variation ( ) over the peripheral areas. Over the plateau, the snowfall rate is low (34 mm yr at 1,200 m above ground level) with a much larger relative seasonal variation ( ). A second study that follows a geographical division highlights the average vertical structure of precipitation and temperature depending on the regions and their interactions with topography. In particular, over ice shelves, we see a strong dependence of the distribution of snowfall on the sea ice coverage. Finally, the relationship between precipitation and temperature is analyzed and compared with a simple analytical relationship. This study highlights that precipitation is largely dependent on the advection of air masses along the topographic slopes with an average vertical wind of 0.02 m s . This provides new diagnostics to evaluate climate models with a three-dimensional approach of the atmospheric structure of precipitation. |
|
| |
Programme |
1013 |
|
| |
Campaign |
|
|
| |
Address |
|
|
| |
Corporate Author |
|
Thesis |
|
|
| |
Publisher |
|
Place of Publication |
|
Editor |
|
|
| |
Language |
|
Summary Language |
|
Original Title |
|
|
| |
Series Editor |
|
Series Title |
|
Abbreviated Series Title |
|
|
| |
Series Volume |
|
Series Issue |
|
Edition |
|
|
| |
ISSN |
2169-8996 |
ISBN |
|
Medium |
|
|
| |
Area |
|
Expedition |
|
Conference |
|
|
| |
Notes |
|
Approved |
yes |
|
| |
Call Number |
|
Serial |
7697 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
Alison Ming, V. Holly L. Winton, James Keeble, Nathan L. Abraham, Mohit C. Dalvi, Paul Griffiths, Nicolas Caillon, Anna E. Jones, Robert Mulvaney, Joël Savarino, Markus M. Frey, Xin Yang |
|
| |
Title |
Stratospheric Ozone Changes From Explosive Tropical Volcanoes: Modeling and Ice Core Constraints |
Type |
Journal |
| |
Year |
2020 |
Publication |
Journal of geophysical research: atmospheres |
Abbreviated Journal |
|
|
| |
Volume |
125 |
Issue |
11 |
Pages |
e2019JD032290 |
|
| |
Keywords |
Antarctica chemistry-climate modeling isotopes in ice cores ozone Samalas volcanic eruption |
|
| |
Abstract |
Major tropical volcanic eruptions have emitted large quantities of stratospheric sulfate and are potential sources of stratospheric chlorine although this is less well constrained by observations. This study combines model and ice core analysis to investigate past changes in total column ozone. Historic eruptions are good analogs for future eruptions as stratospheric chlorine levels have been decreasing since the year 2000. We perturb the preindustrial atmosphere of a chemistry-climate model with high and low emissions of sulfate and chlorine. The sign of the resulting Antarctic ozone change is highly sensitive to the background stratospheric chlorine loading. In the first year, the response is dynamical, with ozone increases over Antarctica. In the high HCl (2 Tg emission) experiment, the injected chlorine is slowly transported to the polar regions with subsequent chemical ozone depletion. These model results are then compared to measurements of the stable nitrogen isotopic ratio, , from a low snow accumulation Antarctic ice core from Dronning Maud Land (recovered in 2016–2017). We expect ozone depletion to lead to increased surface ultraviolet (UV) radiation, enhanced air-snow nitrate photochemistry and enrichment in in the ice core. We focus on the possible ozone depletion event that followed the largest volcanic eruption in the past 1,000 years, Samalas in 1257. The characteristic sulfate signal from this volcano is present in the ice core but the variability in dominates any signal arising from changes in ultraviolet from ozone depletion. Prolonged complete ozone removal following this eruption is unlikely to have occurred over Antarctica. |
|
| |
Programme |
1177 |
|
| |
Campaign |
|
|
| |
Address |
|
|
| |
Corporate Author |
|
Thesis |
|
|
| |
Publisher |
|
Place of Publication |
|
Editor |
|
|
| |
Language |
|
Summary Language |
|
Original Title |
|
|
| |
Series Editor |
|
Series Title |
|
Abbreviated Series Title |
|
|
| |
Series Volume |
|
Series Issue |
|
Edition |
|
|
| |
ISSN |
2169-8996 |
ISBN |
|
Medium |
|
|
| |
Area |
|
Expedition |
|
Conference |
|
|
| |
Notes |
|
Approved |
yes |
|
| |
Call Number |
|
Serial |
7856 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
J. Jumelet, A. R. Klekociuk, S. P. Alexander, S. Bekki, A. Hauchecorne, J. P. Vernier, M. Fromm, P. Keckhut |
|
| |
Title |
Detection of Aerosols in Antarctica From Long-Range Transport of the 2009 Australian Wildfires |
Type |
Journal |
| |
Year |
2020 |
Publication |
Journal of Geophysical Research: Atmospheres |
Abbreviated Journal |
|
|
| |
Volume |
125 |
Issue |
23 |
Pages |
e2020JD032542 |
|
| |
Keywords |
aerosols Antarctica bushfires lidar |
|
| |
Abstract |
We analyze the long-range transport to high latitudes of a smoke particle filament originating from the extratropics plume after the Australian wildfires colloquially known as “Black Saturday” on 7 February and report the first Antarctic stratospheric lidar characterization of such aerosols. Using a high-resolution transport/microphysical model, we show that the monitoring cloud/aerosol lidar instrument operating at the French Antarctic station Dumont d'Urville (DDU, 66°S to 140°E) recorded a signature of those aerosols. The 532 nm scattering ratio of this filament is comparable to typical moderate stratospheric volcanic plume, with values between 1.4 and 1.6 on the first and third days of March above DDU station at around the 14 and 16 km altitude, respectively. A dedicated model is described and its ability to track down fine optical signatures is validated against Antarctic lidar elastic aerosol and DIAL ozone measurements. Using 1 month of tropical Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) data to support a relatively simple microphysical scheme, we report modeled aerosol presence above DDU station after advection of the aerosol size distribution. In situ measurements also report associated positive ozone anomaly. This case study provides evidence that biomass burning events injecting significant amounts of material up to stratospheric altitudes can be transported toward high latitudes. We highlight a potential imprint of smoke particles on the Antarctic atmosphere over larger time scales. Any underestimation of the global impact of such deep particle transport will lead to uncertainties in modeling the associated chemical or radiative effects, especially in polar regions, where specific microphysical and chemical processes take place. |
|
| |
Programme |
209 |
|
| |
Campaign |
|
|
| |
Address |
|
|
| |
Corporate Author |
|
Thesis |
|
|
| |
Publisher |
|
Place of Publication |
|
Editor |
|
|
| |
Language |
|
Summary Language |
|
Original Title |
|
|
| |
Series Editor |
|
Series Title |
|
Abbreviated Series Title |
|
|
| |
Series Volume |
|
Series Issue |
|
Edition |
|
|
| |
ISSN |
2169-8996 |
ISBN |
|
Medium |
|
|
| |
Area |
|
Expedition |
|
Conference |
|
|
| |
Notes |
|
Approved |
yes |
|
| |
Call Number |
|
Serial |
8015 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
Florent Tencé, Julien Jumelet, Slimane Bekki, Sergey Khaykin, Alain Sarkissian, Philippe Keckhut |
|
| |
Title |
Australian Black Summer Smoke Observed by Lidar at the French Antarctic Station Dumont d’Urville |
Type |
Journal |
| |
Year |
2022 |
Publication |
Journal of Geophysical Research: Atmospheres |
Abbreviated Journal |
|
|
| |
Volume |
127 |
Issue |
4 |
Pages |
e2021JD035349 |
|
| |
Keywords |
aerosol Antarctica lidar PSC pyrocumunolimbus stratosphere |
|
| |
Abstract |
In the follow-up of the Australian ”Black Summer” event that persisted from August 2019 to March 2020, we present the optical properties of the stratospheric aerosols injected into the atmosphere by these wildfires. The outbreak of pyrocumulonimbus (PyroCb) activity triggered between 2019/12/29 and 2020/01/04 has raised the stratospheric aerosol load of the Southern Hemisphere to unprecedented levels. Long-range transport brought some of the plumes down to the Antarctic region, where general circulation patterns kept them circling around the continent. The 532 nm Rayleigh/Mie/Raman ground-based lidar of the French Antarctic station Dumont d’Urville (66.6°S–140°E) acquired unprecedented time series of these carbonaceous aerosols starting approximately 20 days after the injection and up to the most recent measurements in October 2019 where local radiosonde reported anomalous ozone depletion as compared to the decadal average. The lidar provides a first and unique time series at high vertical and temporal resolution, complemented by satellite measurements from Ozone Monitoring Instrument, Ozone Mapping and Profiler Suite, and Microwave Limb Sounder. Aerosol backscatter ratio decreases from 1.9 to 1.2 between January and June 2020. Aerosol origin and persistence are characterized, as well as their optical properties and vertical distribution over several months. |
|
| |
Programme |
209 |
|
| |
Campaign |
|
|
| |
Address |
|
|
| |
Corporate Author |
|
Thesis |
|
|
| |
Publisher |
|
Place of Publication |
|
Editor |
|
|
| |
Language |
|
Summary Language |
|
Original Title |
|
|
| |
Series Editor |
|
Series Title |
|
Abbreviated Series Title |
|
|
| |
Series Volume |
|
Series Issue |
|
Edition |
|
|
| |
ISSN |
2169-8996 |
ISBN |
|
Medium |
|
|
| |
Area |
|
Expedition |
|
Conference |
|
|
| |
Notes |
|
Approved |
yes |
|
| |
Call Number |
|
Serial |
8314 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
Jonathan D. Wille, Vincent Favier, Irina V. Gorodetskaya, Cécile Agosta, Christoph Kittel, Jai Chowdhry Beeman, Nicolas C. Jourdain, Jan T. M. Lenaerts, Francis Codron |
|
| |
Title |
Antarctic Atmospheric River Climatology and Precipitation Impacts |
Type |
Journal |
| |
Year |
2021 |
Publication |
Journal of Geophysical Research: Atmospheres |
Abbreviated Journal |
|
|
| |
Volume |
126 |
Issue |
8 |
Pages |
e2020JD033788 |
|
| |
Keywords |
Antarctica atmospheric rivers climatology meteorology |
|
| |
Abstract |
The Antarctic ice sheet (AIS) is sensitive to short-term extreme meteorological events that can leave long-term impacts on the continent's surface mass balance (SMB). We investigate the impacts of atmospheric rivers (ARs) on the AIS precipitation budget using an AR detection algorithm and a regional climate model (Modèle Atmosphérique Régional) from 1980 to 2018. While ARs and their associated extreme vapor transport are relatively rare events over Antarctic coastal regions (∼3 days per year), they have a significant impact on the precipitation climatology. ARs are responsible for at least 10% of total accumulated snowfall across East Antarctica (localized areas reaching 20%) and a majority of extreme precipitation events. Trends in AR annual frequency since 1980 are observed across parts of AIS, most notably an increasing trend in Dronning Maud Land; however, interannual variability in AR frequency is much larger. This AR behavior appears to drive a significant portion of annual snowfall trends across East Antarctica, while controlling the interannual variability of precipitation across most of the AIS. AR landfalls are most likely when the circumpolar jet is highly amplified during blocking conditions in the Southern Ocean. There is a fingerprint of the Southern Annular Mode (SAM) on AR variability in West Antarctica with SAM+ (SAM−) favoring increased AR frequency in the Antarctic Peninsula (Amundsen-Ross Sea coastline). Given the relatively large influence ARs have on precipitation across the continent, it is advantageous for future studies of moisture transport to Antarctica to consider an AR framework especially when considering future SMB changes. |
|
| |
Programme |
411 |
|
| |
Campaign |
|
|
| |
Address |
|
|
| |
Corporate Author |
|
Thesis |
|
|
| |
Publisher |
|
Place of Publication |
|
Editor |
|
|
| |
Language |
|
Summary Language |
|
Original Title |
|
|
| |
Series Editor |
|
Series Title |
|
Abbreviated Series Title |
|
|
| |
Series Volume |
|
Series Issue |
|
Edition |
|
|
| |
ISSN |
2169-8996 |
ISBN |
|
Medium |
|
|
| |
Area |
|
Expedition |
|
Conference |
|
|
| |
Notes |
|
Approved |
yes |
|
| |
Call Number |
|
Serial |
8327 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
A. Barbero, J. Savarino, R. Grilli, C. Blouzon, G. Picard, M. M. Frey, Y. Huang, N. Caillon |
|
| |
Title |
New Estimation of the NOx Snow-Source on the Antarctic Plateau |
Type |
Journal |
| |
Year |
2021 |
Publication |
Journal of Geophysical Research: Atmospheres |
Abbreviated Journal |
|
|
| |
Volume |
126 |
Issue |
20 |
Pages |
e2021JD035062 |
|
| |
Keywords |
Antarctic Plateau flux chamber nitrate photolysis snowpack emissions |
|
| |
Abstract |
To fully decipher the role of nitrate photolysis on the atmospheric oxidative capacity in snow-covered regions, NOx flux must be determined with more precision than existing estimates. Here, we introduce a method based on dynamic flux chamber measurements for evaluating the NOx production by photolysis of snowpack nitrate in Antarctica. Flux chamber experiments were conducted for the first time in Antarctica, at the French-Italian station Concordia, Dome C (75°06'S, 123°20’E, 3233 m a.s.l) during the 2019–2020 summer campaign. Measurements were gathered with several snow samples of different ages ranging from newly formed drifted snow to 6-year-old firn. Contrary to existing literature expectations, the daily average photolysis rate coefficient, , did not significantly vary between differently aged snow samples, suggesting that the photolabile nitrate in snow behaves as a single-family source with common photochemical properties, where a = (2.37 0.35) × 10−8 s−1 (1) has been calculated from December 10th 2019 to January 7th 2020. At Dome C summer daily average NOx flux, , based on measured NOx production rates was estimated to be (4.3 1.2) × 108 molecules cm−2 s−1, which is 1.5–7 times less than the net NOx flux observed previously above snow at Dome C using the gradient flux method. Using these results, we extrapolated an annual continental snow sourced NOx budget of 0.017 0.003 TgN y−1, 2 times the nitrogen budget, (N-budget), of the stratospheric denitrification previously estimated for Antarctica. These quantifications of nitrate photolysis using flux chamber experiments provide a road-map toward a new parameterization of the product that can improve future global and regional models of atmospheric chemistry. |
|
| |
Programme |
1177 |
|
| |
Campaign |
|
|
| |
Address |
|
|
| |
Corporate Author |
|
Thesis |
|
|
| |
Publisher |
|
Place of Publication |
|
Editor |
|
|
| |
Language |
|
Summary Language |
|
Original Title |
|
|
| |
Series Editor |
|
Series Title |
|
Abbreviated Series Title |
|
|
| |
Series Volume |
|
Series Issue |
|
Edition |
|
|
| |
ISSN |
2169-8996 |
ISBN |
|
Medium |
|
|
| |
Area |
|
Expedition |
|
Conference |
|
|
| |
Notes |
|
Approved |
yes |
|
| |
Call Number |
|
Serial |
8393 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
S. Ishino, S. Hattori, M. Legrand, Q. Chen, B. Alexander, J. Shao, J. Huang, L. Jaeglé, B. Jourdain, S. Preunkert, A. Yamada, N. Yoshida, J. Savarino |
|
| |
Title |
Regional Characteristics of Atmospheric Sulfate Formation in East Antarctica Imprinted on 17O-Excess Signature |
Type |
Journal |
| |
Year |
2021 |
Publication |
Journal of Geophysical Research: Atmospheres |
Abbreviated Journal |
|
|
| |
Volume |
126 |
Issue |
6 |
Pages |
e2020JD033583 |
|
| |
Keywords |
aerosols Antarctica isotope methanesulfonate sulfate |
|
| |
Abstract |
17O-excess (Δ17O = δ17O − 0.52 × δ18O) of sulfate trapped in Antarctic ice cores has been proposed as a potential tool for assessing past oxidant chemistry, while insufficient understanding of atmospheric sulfate formation around Antarctica hampers its interpretation. To probe influences of regional specific chemistry, we compared year-round observations of Δ17O of non-sea-salt sulfate in aerosols (Δ17O(SO42−)nss) at Dome C and Dumont d'Urville, inland and coastal sites in East Antarctica, throughout the year 2011. Although Δ17O(SO42−)nss at both sites showed consistent seasonality with summer minima (∼1.0‰) and winter maxima (∼2.5‰) owing to sunlight-driven changes in the relative importance of O3 oxidation to OH and H2O2 oxidation, significant intersite differences were observed in austral spring–summer and autumn. The cooccurrence of higher Δ17O(SO42−)nss at inland (2.0‰ ± 0.1‰) than the coastal site (1.2‰ ± 0.1‰) and chemical destruction of methanesulfonate (MS–) in aerosols at inland during spring–summer (October–December), combined with the first estimated Δ17O(MS–) of ∼16‰, implies that MS– destruction produces sulfate with high Δ17O(SO42−)nss of ∼12‰. If contributing to the known postdepositional decrease of MS– in snow, this process should also cause a significant postdepositional increase in Δ17O(SO42−)nss over 1‰, that can reconcile the discrepancy between Δ17O(SO42−)nss in the atmosphere and ice. The higher Δ17O(SO42−)nss at the coastal site than inland during autumn (March–May) may be associated with oxidation process involving reactive bromine and/or sea-salt particles around the coastal region. |
|
| |
Programme |
1177 |
|
| |
Campaign |
|
|
| |
Address |
|
|
| |
Corporate Author |
|
Thesis |
|
|
| |
Publisher |
|
Place of Publication |
|
Editor |
|
|
| |
Language |
|
Summary Language |
|
Original Title |
|
|
| |
Series Editor |
|
Series Title |
|
Abbreviated Series Title |
|
|
| |
Series Volume |
|
Series Issue |
|
Edition |
|
|
| |
ISSN |
2169-8996 |
ISBN |
|
Medium |
|
|
| |
Area |
|
Expedition |
|
Conference |
|
|
| |
Notes |
|
Approved |
yes |
|
| |
Call Number |
|
Serial |
8412 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
Benjamin Pohl, Vincent Favier, Jonathan Wille, Danielle G Udy, Tessa R Vance, Julien Pergaud, Niels Dutrievoz, Juliette Blanchet, Christoph Kittel, Charles Amory, Gerhard Krinner, Francis Codron |
|
| |
Title |
Relationship Between Weather Regimes and Atmospheric Rivers in East Antarctica |
Type |
Journal |
| |
Year |
2021 |
Publication |
Journal of Geophysical Research: Atmospheres |
Abbreviated Journal |
|
|
| |
Volume |
126 |
Issue |
24 |
Pages |
e2021JD035294 |
|
| |
Keywords |
atmospheric rivers East Antarctica snowfall amounts temperature anomalies weather regimes |
|
| |
Abstract |
Here, we define weather regimes in the East Antarctica—Southern Ocean sector based on daily anomalies of 700 hPa geopotential height derived from ERA5 reanalysis during 1979–2018. Most regimes and their preferred transitions depict synoptic-scale disturbances propagating eastwards off the Antarctic coastline. While regime sequences are generally short, their interannual variability is strongly driven by the polarity of the Southern Annular Mode (SAM). Regime occurrences are then intersected with atmospheric rivers (ARs) detected over the same region and period. ARs are equiprobable throughout the year, but clearly concentrate during regimes associated with a strong atmospheric ridges/blockings on the eastern part of the domain, which act to channel meridional advection of heat and moisture from the lower latitudes towards Antarctica. Both regimes and ARs significantly shape climate variability in Antarctica. Regimes favorable to AR occurrences are associated with anomalously warm and humid conditions in coastal Antarctica and, to a lesser extent, the hinterland parts of the Antarctic plateau. These anomalies are strongly enhanced during AR events, with warmer anomalies and dramatically amplified snowfall amounts. Large-scale conditions favoring AR development are finally explored. They show weak dependency to the SAM, but particularly strong atmospheric ridges/blockings over the Southern Ocean appear as the most favorable pattern, in which ARs can be embedded, and to which they contribute. |
|
| |
Programme |
411 |
|
| |
Campaign |
|
|
| |
Address |
|
|
| |
Corporate Author |
|
Thesis |
|
|
| |
Publisher |
|
Place of Publication |
|
Editor |
|
|
| |
Language |
|
Summary Language |
|
Original Title |
|
|
| |
Series Editor |
|
Series Title |
|
Abbreviated Series Title |
|
|
| |
Series Volume |
|
Series Issue |
|
Edition |
|
|
| |
ISSN |
2169-8996 |
ISBN |
|
Medium |
|
|
| |
Area |
|
Expedition |
|
Conference |
|
|
| |
Notes |
|
Approved |
yes |
|
| |
Call Number |
|
Serial |
8430 |
|
| Permanent link to this record |
| |
|
| |
|
Author |
Meeta Cesler-Maloney, William R. Simpson, Tate Miles, Jingqiu Mao, Kathy S. Law, Tjarda J. Roberts |
|
| |
Title |
Differences in Ozone and Particulate Matter Between Ground Level and 20 m Aloft are Frequent During Wintertime Surface-Based Temperature Inversions in Fairbanks, Alaska |
Type |
Journal |
| |
Year |
2022 |
Publication |
Journal of Geophysical Research: Atmospheres |
Abbreviated Journal |
|
|
| |
Volume |
127 |
Issue |
10 |
Pages |
e2021JD036215 |
|
| |
Keywords |
Alaska inversion ozone PM2.5 pollution vertical |
|
| |
Abstract |
During winter in Fairbanks, Alaska, fine particulate matter (PM2.5) accumulates to large concentrations at breathing level; yet little is known about atmospheric composition aloft. To investigate vertical differences of pollutants, we measured PM2.5 and ozone (O3) at 3 and 20 m above ground level (AGL) in Fairbanks during winter (November 2019–March 2020). We measured temperature and PM2.5 at 3, 6, 9, and 11 m AGL on a tower to quantify surface-based temperature inversions (SBIs) and near-surface PM2.5 gradients. We defined SBIs as data with an 11 m minus 3 m temperature difference greater than 0.5°C. We observed the largest differences in PM2.5 and O3 when SBIs were present. During SBIs, PM2.5 accumulated to large concentrations at 3 m but to a lesser extent at 20 m, demonstrating reduced vertical mixing. During SBIs, the median PM2.5 concentration was 4.8 μg m−3 lower at 20 m than at 3 m. When PM2.5 concentrations were large at 3 m, O3 was often completely chemically removed (titrated) but was still present at 20 m. During SBIs, the O3 mixing ratio was more than 2 nmol mol−1 larger at 20 m than at 3 m in 48% of the data. Results show that during SBIs, pollution in Fairbanks is mixed to altitudes below 20 m AGL and that the oxidation regime of the atmosphere changes from 3 to 20 m AGL as large differences in O3 mixing ratios were measured during SBIs. |
|
| |
Programme |
1215 |
|
| |
Campaign |
|
|
| |
Address |
|
|
| |
Corporate Author |
|
Thesis |
|
|
| |
Publisher |
|
Place of Publication |
|
Editor |
|
|
| |
Language |
|
Summary Language |
|
Original Title |
|
|
| |
Series Editor |
|
Series Title |
|
Abbreviated Series Title |
|
|
| |
Series Volume |
|
Series Issue |
|
Edition |
|
|
| |
ISSN |
2169-8996 |
ISBN |
|
Medium |
|
|
| |
Area |
|
Expedition |
|
Conference |
|
|
| |
Notes |
|
Approved |
yes |
|
| |
Call Number |
|
Serial |
8503 |
|
| Permanent link to this record |
